Ternary fission

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Fission product yields by mass for thermal neutron fission of U-235, Pu-239, a combination of the two typical of current nuclear power reactors, and U-233 used in the thorium cycle ThermalFissionYield.svg
Fission product yields by mass for thermal neutron fission of U-235, Pu-239, a combination of the two typical of current nuclear power reactors, and U-233 used in the thorium cycle

Ternary fission is a comparatively rare (0.2 to 0.4% of events) type of nuclear fission in which three charged products are produced rather than two. As in other nuclear fission processes, other uncharged particles such as multiple neutrons and gamma rays are produced in ternary fission.

Contents

Ternary fission may happen during neutron-induced fission or in spontaneous fission (the type of radioactive decay). About 25% more ternary fission happens in spontaneous fission compared to the same fission system formed after thermal neutron capture, [1] illustrating that these processes remain physically slightly different, even after the absorption of the neutron, possibly because of the extra energy present in the nuclear reaction system of thermal neutron-induced fission.

Quaternary fission, at 1 per 10 million fissions, is also known (see below).

Products

The most common nuclear fission process is "binary fission." It produces two charged asymmetrical fission products with maximally probable charged product at 95±15 and 135±15 u atomic mass. However, in this conventional fission of large nuclei, the binary process happens merely because it is the most energetically probable.

In anywhere from 2 to 4 fissions per 1000 in a nuclear reactor, the alternative ternary fission process produces three positively charged fragments (plus neutrons, which are not charged and not counted in this reckoning). The smallest of the charged products may range from so small a charge and mass as a single proton (Z=1), up to as large a fragment as the nucleus of argon (Z=18).

Although particles as large as argon nuclei may be produced as the smaller (third) charged product in the usual ternary fission, the most common small fragments from ternary fission are helium-4 nuclei, which make up about 90% of the small fragment products. This high incidence is related to the stability (high binding energy) of the alpha particle, which makes more energy available to the reaction. The second-most common particles produced in ternary fission are Tritons (the nuclei of tritium), which make up 7% of the total small fragments, and the third-most are helium-6 nuclei (which decay in about 0.8 seconds to lithium-6). Protons and larger nuclei are in the small fraction (< 2%) which make up the remainder of the small charged products. The two larger charged particles from ternary fission, particularly when alphas are produced, are quite similar in size distribution to those produced in binary fission.

Product energies

The energy of the third much-smaller product usually ranges between 10 and 20 MeV. In keeping with their origin, alpha particles produced by ternary fission typically have mean energies of about ~ 16 MeV (energies this great are never seen in alpha decay). Since these typically have significantly more energy than the ~ 5 MeV alpha particles from alpha decay, they are accordingly called "long-range alphas" (referring to their longer range in air or other media).

The other two larger fragments carry away, in their kinetic energies, the remainder of the fission kinetic energy (typically totalling ~ 170 MeV in heavy element fission) that does not appear as the 10 to 20 MeV kinetic energy carried away by the third smaller product. Thus, the larger fragments in ternary fission are each less energetic, by a typical 5 to 10 MeV, than they are seen to be in binary fission.

Importance

Although the ternary fission process is less common than the binary process, it still produces significant helium-4 and tritium gas buildup in the fuel rods of modern nuclear reactors. [2] This phenomenon was initially detected in 1957, within the environs of the Savannah River National Laboratory. [3]

True ternary fission

A very rare type of ternary fission process is sometimes called "true ternary fission." It produces three nearly equal-sized charged fragments (Z ~ 30) but only happens in about 1 in 100 million fission events. In this type of fission, the product nuclei split the fission energy in three nearly equal parts and have kinetic energies of ~ 60 MeV. True ternary fission has so far only been observed in nuclei bombarded by heavy, high energy ions. [4]

Quaternary fission

Another rare fission process, occurring in about 1 in 10 million fissions, is Quaternary fission. It is analogous to ternary fission, save that four charged products are seen. Typically two of these are light particles, with the most common mode of Quaternary fission apparently being two large particles and two alpha particles (rather than one alpha, the most common mode of ternary fission). [5]

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<span class="mw-page-title-main">Alpha decay</span> Type of radioactive decay

Alpha decay or α-decay is a type of radioactive decay in which an atomic nucleus emits an alpha particle and thereby transforms or 'decays' into a different atomic nucleus, with a mass number that is reduced by four and an atomic number that is reduced by two. An alpha particle is identical to the nucleus of a helium-4 atom, which consists of two protons and two neutrons. It has a charge of +2 e and a mass of 4 Da. For example, uranium-238 decays to form thorium-234.

<span class="mw-page-title-main">Neutron</span> Subatomic particle with no charge

The neutron is a subatomic particle, symbol
n
or
n0
, which has a neutral charge, and a mass slightly greater than that of a proton. Protons and neutrons constitute the nuclei of atoms. Since protons and neutrons behave similarly within the nucleus, and each has a mass of approximately one dalton, they are both referred to as nucleons. Their properties and interactions are described by nuclear physics. Protons and neutrons are not elementary particles; each is composed of three quarks.

<span class="mw-page-title-main">Nuclear physics</span> Field of physics that studies atomic nuclei

Nuclear physics is the field of physics that studies atomic nuclei and their constituents and interactions, in addition to the study of other forms of nuclear matter.

<span class="mw-page-title-main">Nuclear fusion</span> Process of combining atomic nuclei

Nuclear fusion is a reaction in which two or more atomic nuclei, usually deuterium and tritium, combine to form one or more different atomic nuclei and subatomic particles. The difference in mass between the reactants and products is manifested as either the release or absorption of energy. This difference in mass arises due to the difference in nuclear binding energy between the atomic nuclei before and after the reaction. Nuclear fusion is the process that powers active or main-sequence stars and other high-magnitude stars, where large amounts of energy are released.

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Particle radiation is the radiation of energy by means of fast-moving subatomic particles. Particle radiation is referred to as a particle beam if the particles are all moving in the same direction, similar to a light beam.

<span class="mw-page-title-main">Tritium</span> Isotope of hydrogen with two neutrons

Tritium or hydrogen-3 is a rare and radioactive isotope of hydrogen with a half-life of ~12.3 years. The nucleus of tritium contains one proton and two neutrons, whereas the nucleus of the common isotope hydrogen-1 (protium) contains one proton and zero neutrons, and that of hydrogen-2 (deuterium) contains one proton and one neutron.

<span class="mw-page-title-main">Beta particle</span> Ionizing radiation

A beta particle, also called beta ray or beta radiation, is a high-energy, high-speed electron or positron emitted by the radioactive decay of an atomic nucleus during the process of beta decay. There are two forms of beta decay, β decay and β+ decay, which produce electrons and positrons respectively.

<span class="mw-page-title-main">Neutron source</span> Device that emits neutrons

A neutron source is any device that emits neutrons, irrespective of the mechanism used to produce the neutrons. Neutron sources are used in physics, engineering, medicine, nuclear weapons, petroleum exploration, biology, chemistry, and nuclear power.

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Spontaneous fission (SF) is a form of radioactive decay in which a heavy atomic nucleus splits into two or more lighter nuclei. In comparison to induced fission, there is no inciting particle to trigger the decay, it is a purely probabilistic process.

<span class="mw-page-title-main">Nuclear reaction</span> Process in which two nuclei {Nucleus} collide to produce one or more nuclides

In nuclear physics and nuclear chemistry, a nuclear reaction is a process in which two nuclei, or a nucleus and an external subatomic particle, collide to produce one or more new nuclides. Thus, a nuclear reaction must cause a transformation of at least one nuclide to another. If a nucleus interacts with another nucleus or particle and they then separate without changing the nature of any nuclide, the process is simply referred to as a type of nuclear scattering, rather than a nuclear reaction.

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A boosted fission weapon usually refers to a type of nuclear bomb that uses a small amount of fusion fuel to increase the rate, and thus yield, of a fission reaction. The neutrons released by the fusion reactions add to the neutrons released due to fission, allowing for more neutron-induced fission reactions to take place. The rate of fission is thereby greatly increased such that much more of the fissile material is able to undergo fission before the core explosively disassembles. The fusion process itself adds only a small amount of energy to the process, perhaps 1%.

<span class="mw-page-title-main">Neutron activation</span> Induction of radioactivity by neutron radiation

Neutron activation is the process in which neutron radiation induces radioactivity in materials, and occurs when atomic nuclei capture free neutrons, becoming heavier and entering excited states. The excited nucleus decays immediately by emitting gamma rays, or particles such as beta particles, alpha particles, fission products, and neutrons. Thus, the process of neutron capture, even after any intermediate decay, often results in the formation of an unstable activation product. Such radioactive nuclei can exhibit half-lives ranging from small fractions of a second to many years.

<span class="mw-page-title-main">Cluster decay</span> Nuclear decay in which an atomic nucleus emits a small cluster of neutrons and protons

Cluster decay, also named heavy particle radioactivity, heavy ion radioactivity or heavy cluster decay, is a rare type of nuclear decay in which an atomic nucleus emits a small "cluster" of neutrons and protons, more than in an alpha particle, but less than a typical binary fission fragment. Ternary fission into three fragments also produces products in the cluster size. The loss of protons from the parent nucleus changes it to the nucleus of a different element, the daughter, with a mass number Ad = AAe and atomic number Zd = ZZe, where Ae = Ne + Ze. For example:

<span class="mw-page-title-main">Nuclear binding energy</span> Minimum energy required to separate particles within a nucleus

Nuclear binding energy in experimental physics is the minimum energy that is required to disassemble the nucleus of an atom into its constituent protons and neutrons, known collectively as nucleons. The binding energy for stable nuclei is always a positive number, as the nucleus must gain energy for the nucleons to move apart from each other. Nucleons are attracted to each other by the strong nuclear force. In theoretical nuclear physics, the nuclear binding energy is considered a negative number. In this context it represents the energy of the nucleus relative to the energy of the constituent nucleons when they are infinitely far apart. Both the experimental and theoretical views are equivalent, with slightly different emphasis on what the binding energy means.

<span class="mw-page-title-main">Valley of stability</span> Characterization of nuclide stability

In nuclear physics, the valley of stability is a characterization of the stability of nuclides to radioactivity based on their binding energy. Nuclides are composed of protons and neutrons. The shape of the valley refers to the profile of binding energy as a function of the numbers of neutrons and protons, with the lowest part of the valley corresponding to the region of most stable nuclei. The line of stable nuclides down the center of the valley of stability is known as the line of beta stability. The sides of the valley correspond to increasing instability to beta decay. The decay of a nuclide becomes more energetically favorable the further it is from the line of beta stability. The boundaries of the valley correspond to the nuclear drip lines, where nuclides become so unstable they emit single protons or single neutrons. Regions of instability within the valley at high atomic number also include radioactive decay by alpha radiation or spontaneous fission. The shape of the valley is roughly an elongated paraboloid corresponding to the nuclide binding energies as a function of neutron and atomic numbers.

Nuclear fission splits a heavy nucleus such as uranium or plutonium into two lighter nuclei, which are called fission products. Yield refers to the fraction of a fission product produced per fission.

<span class="mw-page-title-main">Alpha particle</span> Helium-4 nucleus; particle of two protons and two neutrons

Alpha particles, also called alpha rays or alpha radiation, consist of two protons and two neutrons bound together into a particle identical to a helium-4 nucleus. They are generally produced in the process of alpha decay but may also be produced in other ways. Alpha particles are named after the first letter in the Greek alphabet, α. The symbol for the alpha particle is α or α2+. Because they are identical to helium nuclei, they are also sometimes written as He2+
or 4
2
He2+
indicating a helium ion with a +2 charge. Once the ion gains electrons from its environment, the alpha particle becomes a normal helium atom 4
2
He
.

References

  1. https://web-docs.gsi.de/~wolle/FISSION/ternary/ternary.html Fraction ternary fission as a function of different Z and A in fissile isotopes.
  2. Comparative study of the ternary particle emission in 243-Cm (nth,f) and 244-Cm(SF). S. Vermote, et al. inDynamical aspects of nuclear fission: proceedings of the 6th International Conference. Ed. J. Kliman, M. G. Itkis, S. Gmuca. World Scientific Publishing Co. Pte. Ltd. Singapore. (2008)
  3. Discovery That Nuclear Fission Produces Tritium Edward L. Albenesius, J. Henry Horton Harold M. Kelley, Daniel S. St. John, and Robert S. Ondrejcin
  4. "True ternary fission". January 2003.
  5. Ternary and Quaternary fission